Abstract:
We report the transport and magnetic properties of La-deficient ultrathin films of La1-8MnO3 (LMO) grown on SrTiO3 (STO) and engineered by using different interfacial layers. LMO layer and adjusting interface oxide (LaO-STO and SMO) layers were grown by a metalorganic aerosol deposition technique with monolayer accuracy. The role of LaO-TiO2 interface in the formation of ferromagnetic metallic state in very thin LMO films was demonstrated. Ferromagnetic metallic ground state in LMO films with the thickness down to 6 monolayers is stabilized by a combination of a La-deficiency and the interface-induced doping.